Researchers electrically manipulate a ‘chiral interface state’ in a 2D material

Researchers from  Purdue University, University of California, Lawrence Berkeley National Laboratory and Japan's National Institute for Materials Science have managed to electrically manipulate a ‘chiral interface state’ in twisted monolayer-bilayer graphene, with potential for energy-efficient microelectronics and quantum computing.

The international research team, led by Lawrence Berkeley National Laboratory (Berkeley Lab), has taken the first atomic-resolution images and demonstrated electrical control of a chiral interface state – an exotic quantum phenomenon that could help researchers advance quantum computing and energy-efficient electronics.


The chiral interface state is a conducting channel that allows electrons to travel in only one direction, preventing them from being scattered backwards and causing energy-wasting electrical resistance. Researchers are working to better understand the properties of chiral interface states in real materials but visualizing their spatial characteristics has proved to be exceptionally difficult.

Now, for the first time, atomic-resolution images captured by the research team have directly visualized a chiral interface state. The researchers also demonstrated on-demand creation of these resistance-free conducting channels in a 2D insulator. Their work is part of Berkeley Lab’s broader push to advance quantum computing and other quantum information system applications, including the design and synthesis of quantum materials to address pressing technological needs.

“Previous experiments have demonstrated that chiral interface states exist, but no one has ever visualized them with such high resolution. Our work shows for the first time what these 1D states look like at the atomic scale, including how we can alter them – and even create them,” said first author Canxun Zhang, a former graduate student researcher in Berkeley Lab’s Materials Sciences Division and the Department of Physics at UC Berkeley. He is now a postdoctoral researcher at UC Santa Barbara.

Chiral interface states can occur in certain types of 2D materials known as quantum anomalous Hall (QAH) insulators that are insulators in bulk but conduct electrons without resistance at one-dimensional “edges” – the physical boundaries of the material and interfaces with other materials.

To prepare chiral interface states, the team worked at Berkeley Lab’s Molecular Foundry to fabricate a device called twisted monolayer-bilayer graphene, which is a stack of two atomically thin layers of graphene rotated precisely relative to one another, creating a moiré superlattice that exhibits the QAH effect.

In subsequent experiments at the UC Berkeley Department of Physics, the researchers used a scanning tunneling microscope (STM) to detect different electronic states in the sample, allowing them to visualize the wavefunction of the chiral interface state. Other experiments showed that the chiral interface state can be moved across the sample by modulating the voltage on a gate electrode placed underneath the graphene layers. In a final demonstration of control, the researchers showed that a voltage pulse from the tip of an STM probe can “write” a chiral interface state into the sample, erase it, and even rewrite a new one where electrons flow in the opposite direction.

The findings could help researchers build tunable networks of electron channels with promise for energy-efficient microelectronics and low-power magnetic memory devices in the future, and for quantum computation making use of the exotic electron behaviors in QAH insulators.

The researchers intend to use their technique to study more exotic physics in related materials, such as anyons, a new type of quasiparticle that could enable a route to quantum computation.

“Our results provide information that wasn’t possible before. There is still a long way to go, but this is a good first step,” Zhang said.

Posted: Apr 11,2024 by Roni Peleg